Go to View --> ToolBox --> And you can add any controls.Or else you can add a bit of code as below.
<Button Content="Click Me" HorizontalAlignment="Left" Margin="138,161,0,0" VerticalAlignment="Top" RenderTransformOrigin="0.617,1.507" Height="117" Width="190" Click="Button_Click_1"/>Then to add click action for controls you can just double click the controls and you may navigate to xaml.cs page where you can add your code.
 
namespace AddControls
{
    public partial class MainPage : PhoneApplicationPage
    {
        // Constructor
        public MainPage()
        {
            InitializeComponent();
            // Sample code to localize the ApplicationBar
            //BuildLocalizedApplicationBar();
        }
        private void Button_Click_1(object sender, RoutedEventArgs e)
        {
            Console.WriteLine("Iam being Clicked......");
        }
nice..
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